Laser induced incandescence measurements of soot volume fraction and effective particle size in a laminar co-annular non-premixed methane/air flame at pressures between 0.5–4.0 MPa

Publication Type  Journal Article
Year of Publication  2006
Authors  Thomson, K.A.; Snelling, D.R.; Smallwood, G.J.; Liu, F.
Journal Title  Applied Physics B: Lasers and Optics
Volume  83
Issue  3
Pages  469 - 475
Journal Date  06/2006
Abstract  An auto-compensating laser-induced incandescence (AC-LII) technique was applied for the first time to measure soot volume fraction (SVF) and effective primary particle diameter (dpeff) in a high pressure methane/air non-premixed flame. The measured dpeff profiles had annular structures and radial symmetry, and the particle size increased with increasing pressure. LII-determined SVFs were lower than those measured by a line of sight attenuation (LOSA) technique. The LOSA measured soot volume fractions were corrected for light scattering using the Rayleigh–Debye–Gans polydisperse fractal aggregate (RDG-PFA) theory, the dpeff data, and assumptions regarding the soot aggregate size distribution. The correction dramatically improved agreement between data obtained using these two measurement techniques. Qualitatively, soot volume distributions obtained using LII had more annular shapes than those obtained using LOSA. Nonetheless, it has been demonstrated that the AC-LII technique is very well suited for application in media where attenuation of the excitation laser pulse energy can exceed 45%. This paper also underlines the importance of correcting LOSA SVF measurements for light scattering in high pressure flames.
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